I quite enjoy the soundtrack of the Dean Martin/Jerry Lewis-film Sailor Beware, with songs such as Sailor Polka, Old Calliope, Today, Tomorrow, Forever and Never Before.
I also LOVE the soundtrack of A Hard Day's Night and Help!
I also think the movies Love Me Tender and Jailhouse Rock have an excellent soundtrack.
And what about the title song of the James Bond-film Live And Let Die? Also marvelous.
And the title song of Ocean's Eleven (1960) , that is called Eee O Eleven, that is sung by Sammy Davis Jr. is also perfect.